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This two record set, released by Capitol in 1969 covers all the bases; Witches, black magic, demons, how to make a pact with the devil and more. It also describes the burning of witches and spellcasting in incredibly graphic detail. This album, even at 45 years old, is definitely not for the squeamish.
Also see: Halloween Hits: Sounds of Terror! - Pickwick Records (1974) and Halloween Hits: Chilling, Thrilling Sounds of The Haunted House - Disneyland Records (1964)